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To Make the Cacao Nib Pastry Dough:
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Position a rack in the center of the oven and preheat the oven to 350F.
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Spray the inside of each tartlet pan with nonstick baking spray and place the pans on a baking sheet.
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Place the walnuts in a cake or pie pan and toast in the oven for 7 to 8 minutes, until light golden.
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Remove the pan from the oven and cool on a rack.
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Chop the walnuts finely.
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Pulse together the flour, brown sugar, and salt in the work bowl of a food processor fitted with a steel blade.
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Cut the butter into small pieces and add it to the flour mixture.
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Pulse until the butter is cut into very tiny pieces, about 30 seconds.
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The texture will be sandy with very tiny lumps throughout.
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Add the cacao nibs and chopped walnuts and pulse briefly to blend.
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In a small bowl, use a fork to beat the egg yolk and vanilla together.
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With the food processor running, pour this mixture through the feed tube.
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Process the dough until the mixture wraps itself around the blade, about 1 minute.
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Break off walnut-size pieces of the dough and press them into the tartlet pans.
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Pinch off any excess dough at the top edge of the pans.
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Place another tartlet pan on top of each tartlet to act as a weight while it bakes.
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Bake the tartlet shells for 7 minutes.
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Remove the top tartlet pans.
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If the bottoms of the pastry shells puff up, gently pierce them with a fork or the point of a knife to release the air.
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Bake another 7 to 8 minutes, until light golden and set.
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Remove the baking sheet from the oven and transfer it to a rack to cool completely.
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To remove the tartlet shells from their pans, gently tap each pan on the countertop.
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To Make the Ganache Filling:
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Place the chopped chocolate in a 2-quart bowl.
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Place the cream in a medium saucepan and bring to a boil over medium heat.
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Pour the cream over the chocolate.
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Let it stand for 15 seconds, then stir together with a rubber spatula, whisk, or immersion blender until very smooth.
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To Assemble:
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Use a 1-inch round ice cream scoop to fill each tartlet shell to the top with ganache.
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Chill for 15 minutes to set the filling, or let it set at room temperature for 30 minutes to 1 hour.
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Serve at room temperature.
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Keeping:
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Store the tartlets in a single layer on a baking sheet.
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Cover the tops of the tartlets with a large piece of waxed paper to keep the surface from becoming marred.
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Tightly wrap the pan with aluminum foil and keep in the refrigerator up to 3 days.
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Streamlining:
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The pastry dough can be made in advance and kept in the refrigerator, tightly wrapped in a double layer of plastic wrap, up to 4 days before using.
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To freeze up to 4 months, wrap it in a double layer of plastic wrap and enclose it in a freezer bag.
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Use a large piece of masking tape and an indelible marker to label and date the contents.
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If frozen, defrost the dough in the refrigerator overnight before using.
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If it is too cold to roll out, let it stand at room temperature to become pliable.
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The tartlet shells can be baked and held at room temperature up to 2 days before filling.
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After they are completely cool, place them on a jelly-roll pan, cover with waxed paper, and tightly wrap the pan in aluminum foil.